eprintid: 3146 rev_number: 11 eprint_status: archive userid: 387 dir: disk0/00/00/31/46 datestamp: 2018-11-15 09:20:18 lastmod: 2018-11-15 09:20:18 status_changed: 2018-11-15 09:20:18 type: article metadata_visibility: show creators_name: Joe, Sung-yoon creators_name: Ryu, Shinyoung creators_name: Nguyen, Duc Cuong creators_name: Yim, Jong Hyuk creators_name: Jeong, Huiseong creators_name: Ha, Na Young creators_name: Ahn, Y.H. creators_name: Park, Ji-Yong creators_name: Lee, Soonil creators_id: cuongnd@vnu.edu.vn creators_id: soonil@ajou.ac.kr title: Contributions of poly(3-hexylthiophene) nanowires to alteration of vertical inhomogeneity of bulk-heterojunction active layers and improvements of light-harvesting and power-conversion efficiency of organic solar cells ispublished: pub subjects: Scopus subjects: isi divisions: fac_physic abstract: We report a 47.1% efficiency improvement resulting from the combination of device-architecture modification and inclusion of poly(3-hexylthiophene-2,5-diyl) nanowires (P3HT NWs) in bulk heterojunction (BHJ) active layers (ALs). Modelling of ellipsometry spectra shows substantial changes in inhomogeneity and optical constants of BHJ ALs with P3HT-NW inclusion. Furthermore, finite-difference time-domain simulation results based on actual device structures with inhomogeneous AL models indicate that enhanced light harvesting is a main contributing factor to efficiency improvement. On the contrary, P3HT-NW inclusion has no significant effect on charge carrier collection, other than suppressing occurrence of cul-de-sac in hole-transport pathways and unfavourable indene-C60 bisadduct domains near top anodes. date: 2017-01-03 date_type: published publisher: Elsevier B.V. official_url: https://www.elsevier.com/en-xs id_number: 10.1016/j.orgel.2016.12.063 full_text_status: public publication: Organic Electronics volume: 42 pagerange: 372-378 refereed: TRUE issn: 1566-1199 citation: Joe, Sung-yoon and Ryu, Shinyoung and Nguyen, Duc Cuong and Yim, Jong Hyuk and Jeong, Huiseong and Ha, Na Young and Ahn, Y.H. and Park, Ji-Yong and Lee, Soonil (2017) Contributions of poly(3-hexylthiophene) nanowires to alteration of vertical inhomogeneity of bulk-heterojunction active layers and improvements of light-harvesting and power-conversion efficiency of organic solar cells. Organic Electronics, 42 . pp. 372-378. ISSN 1566-1199 document_url: https://eprints.uet.vnu.edu.vn/eprints/id/eprint/3146/1/Organic%20Electronics%2042%20%282017%29%20372-378.pdf